Process Intensification of CO2 Desorption

dc.authorid0000-0003-4191-4960
dc.authorid0000-0002-1950-4538
dc.contributor.authorGecim, Gozde
dc.contributor.authorOuyang, Yi
dc.contributor.authorRoy, Sangram
dc.contributor.authorHeynderickx, Geraldine J.
dc.contributor.authorVan Geem, Kevin M.
dc.date.accessioned2026-02-12T21:05:11Z
dc.date.available2026-02-12T21:05:11Z
dc.date.issued2022
dc.departmentBursa Teknik Üniversitesi
dc.description.abstractAnthropogenic climate change due to, among other causes, unhindered CO2 emissions is a major concern worldwide. The post combustion capture (PCC) process using a solvent, known as chemical absorption, is currently the most effective way to reduce CO2 emissions from large point sources. However, high capital investment costs when using the conventional packed bed absorber/desorber technology and high energy requirements during solvent regeneration are the primary obstacles for its large-scale implementation. Different process intensification (PI) technologies to desorb CO2 from the solvent have been introduced to mitigate the energy consumption compared to the conventional packed bed technology. This work reviews different technologies for intensification of CO2 desorption. In this context, rotating packed beds, microreactors, and membrane contactors have been explored as potential alternatives to intensify the desorption because of their superior mass and heat transfer. Alternative energy sources like ultrasound and microwaves have also been used to improve the desorption performance of conventional equipments. PI can also be realized by using novel solvents with improved desorption kinetics in combination with intensification equipment. Thus in this review, a comprehensive assessment of different existing PI technologies based on regeneration energies and regeneration efficiencies relative to conventional technology is presented. The intensification of mass transfer for the different technologies is compared, and a new parameter, named the regeneration factor, is proposed to evaluate the performance of PI equipment. This study outlines the advances in process intensification of CO2 desorption technologies to date and presents an overview of the merits and limits of all technologies.
dc.description.sponsorshipTUBITAK; Research Foundation - Flanders (FWO) [1273421N]; Flemish Government; Flanders Innovation AMP; Entrepreneurship (VLAIO) [HBC.2021.0255]; European Research Council under the European Union [818607]
dc.description.sponsorshipG.G. thanks TUBITAK for 2214-A International Research Fellowship Programme for Ph.D. Students. Y.O. gratefully acknowledges financial support from a postdoctoral fellowship from the Research Foundation - Flanders (FWO) Grant Number 1273421N. We gratefully acknowledge the financial support of the Flemish Government and Flanders Innovation & Entrepreneurship (VLAIO) through the Moonshot project CAPTIN-2 (HBC.2021.0255). In addition, the research leading to these results received funding from the European Research Council under the European Union's Horizon 2020 research and innovation programme/ERC Grant Agreement No. 818607.
dc.identifier.doi10.1021/acs.iecr.2c01689
dc.identifier.endpage19196
dc.identifier.issn0888-5885
dc.identifier.issn1520-5045
dc.identifier.issue45
dc.identifier.scopus2-s2.0-85137892521
dc.identifier.scopusqualityQ1
dc.identifier.startpage19177
dc.identifier.urihttps://doi.org/10.1021/acs.iecr.2c01689
dc.identifier.urihttps://hdl.handle.net/20.500.12885/6838
dc.identifier.volume62
dc.identifier.wosWOS:000851046200001
dc.identifier.wosqualityQ2
dc.indekslendigikaynakWeb of Science
dc.indekslendigikaynakScopus
dc.language.isoen
dc.publisherAmer Chemical Soc
dc.relation.ispartofIndustrial & Engineering Chemistry Research
dc.relation.publicationcategoryMakale - Uluslararası Hakemli Dergi - Kurum Öğretim Elemanı
dc.rightsinfo:eu-repo/semantics/openAccess
dc.snmzKA_WoS_20260212
dc.subjectCarbon-Dioxide Capture
dc.subjectCatalytic Solvent Regeneration
dc.subjectCo2-Loaded Mea Solution
dc.subjectMonoethanolamine Aqueous-Solutions
dc.subjectMass-Transfer Rates
dc.subjectPilot-Plant
dc.subjectStripper Configurations
dc.subjectAlkanolamine Solutions
dc.subjectHeat Duty
dc.subject2-Amino-2-Methyl-1-Propanol Amp
dc.titleProcess Intensification of CO2 Desorption
dc.typeArticle

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