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Öğe Characterization of CdS films and CdS/Si heterojunctions prepared by ultrasonic spray pyrolysis and their response to light(Elsevier, 2020) Bilgin, Vildan; Sarıca, Emrah; Demirselcuk, Barbaros; Erturk, KadirIn this work CdS thin films were deposited onto glass and p-Si substrates by ultrasonically spraying of precursor solutions prepared in molarity ranging from 0.025 M, to 0.1 M. Structural investigations revealed that all films have hexagonal structure and mean crystallite size was found to be in the range of 18 nm-21 nm. On the other hand, CdS films exhibited 65-70% optical transmittance and band gap energy for all films was found to be about 2.42 eV. Electrical measurements of CdS/Si heterojunctions were carried out under both dark and illumination conditions. Calculated ideality factor and zero-bias barrier height ranged from 3.02 to 2.66 and 0.74 eV-0.78 eV according to TE theory whereas they ranged from 6.91 to 4.73 and 0.71 eV-0.74 eV according to Cheungs' method. Increase in reverse saturation current when heterojunctions were illuminated indicated that they have good sensitivity to solar light.Öğe Iron doped ZnO thin films deposited by ultrasonic spray pyrolysis: structural, morphological, optical, electrical and magnetic investigations(Springer, 2018) Bilgin, Vildan; Sarıca, Emrah; Demirselcuk, Barbaros; Turkyilmaz, SerenIn this work, undoped and Fe-doped ZnO thin films at various concentrations (2, 4 and 6 at.%) were deposited onto glass substrate by using ultrasonic spray pyrolysis in order to investigate the effect of Fe doping on the structural, morphological, optical, electrical and magnetic properties of ZnO thin films. X-ray diffractometer (XRD) results revealed that all deposited thin films have hexagonal wurtzite structure and Fe doping led to decrease in mean crystallite size. Atomic force microscopy images showed that thin films were composed of tightly packed grains. Optical examinations indicated that optical transmittance remarkably decreased with the increase in the amount of Fe concentration in thin films. Additionally, optical band gap of deposited films were determined in the range of 3.26-3.29 eV. It was determined that all deposited thin films have n-type conductivity and electrical resistivity increased up to 253.6 Omega cm as a consequence of Fe doping. Vibrating sample magnetometer measurements showed that all films have ferromagnetic behavior.Öğe Ultrasonically sprayed cobalt oxide thin films: Enhancing of some physical properties by nickel doping(Elsevier B.V., 2021) Kus, Esra; Kucukarslan, Ayse; Demirselcuk, Barbaros; Sarıca, Emrah; Akyuz, Idris; Bilgin, VildanIn this study, the effect of Ni doping (3, 6, 9 at%) on structural, optical, electrical and magnetic properties of Co3O4 films was reported. Films were grown at 300 ± 5 °C substrate temperature via ultrasonic spray pyrolysis (USP) technique. The structural analyses showed that undoped and Ni (3%) doped films exhibit an amorphous structure. Ni doping at higher ratios caused the films to have improved crystallinity. Optical band gap values the films were found to be between 2.03 and 2.08 eV with an additional sub-band corresponding to energies varying between 1.35 and 1.46 eV. The electrical conductivity values of the films increased significantly depending on the Ni doping. The hysteresis curves of the films showed that the films have weak ferromagnetic properties. Ni doping significantly improved the structural and electrical properties of Co3O4 films making them suitable materials for technological applications.